Love Missionary's approach. Remove all the variables and then work backwards. I think the lever guns get a bad wrap when it is really not the action type that causes the problems, but other issues. I read almost all the posts here so let's list what has been brought up.
Twist rate is meant for a short, slow bullet.
Dovetail cuts can cause tight spots in the bore.
Forend it touching the barrel
Ammo moving inside the magazine tube changing recoil direction
Various attachments, mag tube, forend band, muzzle band all in some form of contact with the barrel.
Goofy scope
So, here is my 2 cents worth (probably worth about 1.2 cents in reality) on the subject.
First, I suspect that Marlin chose the slow twist because they knew that lead bullets would get shot in the rifle and being micro-groove, a faster twist might just strip out on fast moving lead bullets. So, to the points made by others, slow down the bullet and reduce the size to something like a .44-40 slug. I would lean towards a softer alloy like 20:1 or even 30:1 and prefer a true PB bullet to assure a good seal, and not a bevel-base bullet.
At this point, although this is a lever gun with a tubular mag, I would not use a crimp. I would simply use about 0.002 neck tension while you are trying to get the rifle to shoot. A crimp is just another variable that is not easy to control. If your crimp is not uniform, unless you mark the cases and index them in the press and when chambering them, a non-uniform crimp will be randomly positioned in the chamber for every shot.
Nobody has mentioned the muzzle crown. Looking at your targets, I see no pattern to any of the groups, regardless of size. They seem to be very random. There is one exception, two targets have a cluster of 3 or so at the top and then two flyers down below. The rest are pretty random. That would make me think that the crown on the muzzle needs some work. If there is a slight burr, it will tear the bullet and more than likely cause erratic departure from the muzzle along with erratic flight. I would check the crown with a 10x loupe and if at all in doubt, make a brass lap and make sure the crown is perfect. I'm not talking about angularity here. That will create a consistent change in point of impact. I'm talking about a burr, raised area and such from the machining process.
Next, I would try Missionary's suggestion of stripping down the rifle to just the barrel and action. Always rest the barrel in the same spot on your bag. Even if you don't get the load right, if you use a smaller bullet at reduced velocities, at 50 yds you should be able to shoot a decent sized group. Even if you took the scope off (to remove that variable) you should be able to shoot a decent group at 50 yds with iron sights assuming that you don't have geezer eyes and can shoot iron sights. If the rifle will not shoot stripped down to its basic parts, then you need to look deeper. Running a slug down the bore to check for tight spots would probably be my next move. I'd lap the barrel with JB Bore paste while I was at it. Then if there are no high spots, no muzzle burrs and your scope is proven good, I would pick a powder like 2400 or Unique and do a ladder test using the same short, light bullet. I'd start with 1/2 grain increments. And as much as I love 2400, I might hold off and stay with faster pistol powders given the reduced velocity. You want a harder smack in the ass to have the PB fill the bore and seal rather than a push from a magnum type powder.
And that last point brings up one last though. If you have a GC bullet you can shoot in the rifle, I'd give that a try to see if it makes a difference. If it will shoot well with a GC bullet, then it's telling you that you need to find the sweet spot to shoot a PB bullet.